TY - JOUR AU - An, Yanqing AU - Xu, Jianzhong AU - Feng, Lin AU - Zhang, Xinghua AU - Liu, Yanmei AU - Kang, Shichang AU - Jiang, Bin AU - Liao, Yuhong PY - 2019 DA - 2019// TI - Molecular characterization of organic aerosol in the Himalayas: insight from ultra-high-resolution mass spectrometry JO - Atmospheric Chemistry and Physics VL - 19 IS - 2 CY - State Key Laboratory of Cryospheric Science, Northwest Institute ofEco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000,China;;State Key Laboratory of Organic Geochemistry, Guangzhou Institute ofGeochemistry, Chinese Academy of Sciences, Guangzhou 510640, China;;University of Chinese Academy of Sciences (UCAS), Beijing 100049,China AB - An increased trend in aerosol concentration has been observed in theHimalayas in recent years, but the understanding of the chemical compositionand sources of aerosol remains poorly understood. In this study, molecularchemical composition of water-soluble organic matter (WSOM) from two filtersamples collected during two high aerosol loading periods (denoted as P1 andP2) at a high-altitude station (Qomolangma Station, QOMS;4276  m  a.s.l.) in the northern Himalayas was identified usingelectrospray ionization Fourier transform ion cyclotron resonance massspectrometry (ESI-FTICR MS). More than 4000 molecular formulas wereidentified in each filter sample which were classified into two compoundgroups (CHO and CHON) based on their elemental composition, with bothaccounting for nearly equal contributions in number (45 %–55 %).The relative abundance weighted mole ratio of O∕Cw for P1 and P2was 0.43 and 0.39, respectively, and the weighted double bond equivalents(DBE w... SN - 1680-7324 ID - An2019 ER -